If you mean - you want to sync a specific SQL CE 3.5 database (on one machine) to a SQL server 2005 or 2008 on a different machine, then you should be able to do it. LocalDatabase Cache is a SQL CE database for example.
However, before you create an App to do the sync, you may want to back up your local data on the SQL CE 3.5 database somewhere else if this is your first time to write a sync app.
Thanks.
Leo Zhou
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